Authors Li, J; Xu, Y; Wang, S; Zhang, H in AMER CHEMICAL SOC published article about SUPPORTED GOLD NANOPARTICLES; SELECTIVE OXIDATION; PD; PALLADIUM; CATALYST; CO; STABILIZATION; DFT in [Li, Jin; Xu, Yang; Wang, Shuai; Zhang, Hui] Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, POB 98, Beijing 10029, Peoples R China in 2019.0, Cited 49.0. Name: Benzyl Alcohol. The Name is Benzyl Alcohol. Through research, I have a further understanding and discovery of 100-51-6
A series of Ni3Al-LDH-supported AuPd nanocluster (NC) catalysts AuxPdy/LDH (x/y = Au/Pd ratio upon the molar percentages of Au and Pd to the total metal; LDH: layered double hydroxide) were prepared by modified electrostatic adsorption of captopril-protected AuxPdy NCs onto the predispersed LDH support followed by proper calcination. The systematic characterizations reveal that the ultrafine AuxPdy NCs ranging from 1.4 +/- 0.5 to 1.6 +/- 0.5 nm with the Au/Pd ratios reducing from 96/4 to 61/39 are mainly dispersed on the edge of small LDH nanosheets in obtained catalysts AuxPdy/LDH. All of the catalysts AuxPdy/LDH exhibit higher aerobic oxidation activity of 1-phenylethanol than the monometallic Au-25/LDH, of which the Au87Pd13/LDH (1.5 +/- 0.5 nm) shows the highest activity with turnover frequency (TOF) of 6810 h(-1) in toluene and an extremely high performance with 131 400 h(-1) under solvent-free condition, attributed to the ultrasmall Au87Pd13 NCs, the most electron-rich Au species formed by the electron transfer from Pd to Au and Ni-OH to Au87Pd13 NCs and the strongest Au87Pd13 NCs-LDH synergistic effect. Moreover, the catalyst maintains 98% of the initial conversion of 1-phenylethanol after 10 runs and possesses good adaptability for substrate alcohols.
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Reference:
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,Preparation of Indole Containing Building Blocks for the Regiospecific Construction of Indole Appended Pyrazoles and Pyrroles